Plasmon-Enhanced Solar-Driven Hydrogen Evolution Using Titanium Nitride Metasurface Broadband Absorbers

نویسندگان

چکیده

Broadband perfect absorbers in the visible region have attracted considerable attention many fields, especially solar thermophotovoltaic and energy harvesting systems. However, developing light with high absorptivity, thermal stability, a broad bandwidth remains great challenge. Here, we theoretically experimentally demonstrate that titanium nitride metasurface absorber exhibits broadband absorption an average of more than 92% over wavelength range 400 to 750 nm. The increase is attributed localized surface plasmon resonance (LSPR). We plasmon-enhanced visible-light-driven hydrogen production from water using polymer photocatalyst integrated TiN absorber. A 300% evolution rate was observed due LSPR enhances rates absorption, carrier separation, hot-carrier transfer photocatalyst. These results enable new approach prepare high-efficiency

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ژورنال

عنوان ژورنال: ACS Photonics

سال: 2021

ISSN: ['2330-4022']

DOI: https://doi.org/10.1021/acsphotonics.1c00927